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Highlights from 4 Papers in 2022

In 2022, Jaffe Group members authored or co-authored 7 papers. Here are highlights from 4:

1.            Sedlacek  A.J. Lewis E.R., Onasch T.B., Zuidema P., Redemann J., Jaffe D, and Kleinman L.I. “Using the Black Carbon Particle Mixing State to Characterize the Lifecycle of Biomass Burning Aerosols.” Environmental Science & Technology, 56 (20), 14315-14325, http://10.1021/acs.est.2c03851, 2022.

In this analysis, a team, led by Art Sedlacek at Brookhaven National Lab, used data from the Mt. Bachelor Observatory and other sites to show how secondary organic aerosols and black carbon change as wildfire smoke ages.  This work has important implications for the climate forcing of smoke.

2.            Jaffe, D. A., Schnieder, B., and Inouye, D. “Technical note: Use of PM2.5 to CO ratio as an indicator of wildfire smoke in urban areas.” Atmos. Chem. Phys., 22, 12695–12704, https://doi.org/10.5194/acp-22-12695-2022, 2022.

In this analysis, Dan and coauthors show how the PM2.5/CO ratio can be used to track wildfire smoke in urban locations.

3.            Jaffe, D. A., Ninneman, M., & Chan, H. C. “NOx and O3 trends at U.S. non-attainment areas for 1995–2020: Influence of COVID-19 reductions and wildland fires on policy-relevant concentrations.” Journal of Geophysical Research: Atmospheres, 127, e2021JD036385. https://doi.org/10.1029/2021JD036385, 2022.

In this analysis, Dan and coauthors examined data from 32 Nonattainment areas in the US (cities that fail to meet the US ozone standard) to better understand the relationship between nitrogen oxides (mainly from vehicles) and Ozone.  The analysis showed how ozone was reduced in 2020 in the Eastern U.S. (due to COVID-19 related traffic reductions) but increased in the Western U.S. due to the large number and area of wildfires burning that year.

4.            Bernays, N., Jaffe, D. A., Petropavlovskikh, I., and Effertz, P. Comment on “Comparison of ozone measurement methods in biomass burning smoke: an evaluation under field and laboratory conditions” by Long et al. Atmos. Meas. Tech., 15, 3189–3192, https://doi.org/10.5194/amt-15-3189-2022, 2022.

In this analysis, Jaffe-group team member Noah Bernays and coauthors confirmed a significant interference in the measurement of O3 in smoke for some UV instruments. This interference was attributed to the use of manganese chloride as the scrubber material, for example in the Thermo Fisher’s 49i series ozone analyzers. Instruments employing manganese dioxide scrubbers did not show this interference.